TBH I want to vote negative for all the Narutos & One Piece, but a lot of you seem to like those kinds of anime I spose.
Here's some popular ones just cause of TV but I'd say popular animes are still a must to know bout.
Samurai Champloo
Cowboy Bebop
Trigun
.Hack//Sign
Wolf's Rain
For movies anything from that Spirited Away guy is def good.
5 Centimeters Per Second - majorly sad
The Girl Who Leapt Through Time -sad
Ouran High School Host Club lol. ;c
Chobits
Lovely Complex
Elfen Lied
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